T9 Advances in Understanding Aquifer Heterogeneity and Multi-Scale Flow and Transport in Porous and Fractured Media
Sunday, 31 October 2010
8:00 AM - 12:00 PM
Room 612
COUPLED-PROCESS MODELING OF IN SITU URANIUM BIOREMEDIATION NEAR RIFLE, COLORADO
Paper number: T9-3
Program: Technical Sessions
Time: 8:20 AM – 8:35 AM
Authors
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Steven B. YabusakiPacific Northwest National Laboratory, Richland, WA
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Yilin FangPacific Northwest National Laboratory, Richland, WA
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Scott R. WaichlerPacific Northwest National Laboratory, Richland, WA
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Yi-Ju BottPacific Northwest National Laboratory, Richland, WA
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Andy WardPacific Northwest National Laboratory, Richland, WA
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Philip LongPacific Northwest National Laboratory, Richland, WA
Abstract
A fully 3-D reactive transport model integrating abiotic and microbially mediated reactions has been developed to simulate biostimulation field experiments at a former Uranium Mill Tailings Remedial Action (UMTRA) site near Rifle, Colorado. Indicator simulations of lithofacies were combined with property transfer models to generate realizations of facies-specific hydrologic parameters (e.g., hydraulic conductivity, porosity, surface area) based on lithologic logs, slug tests, electromagnetic borehole flowmeter measurements, particle size distributions, and measurements of surface area. The 3-D reactive transport model includes variably saturated flow and a comprehensive reaction network (102 biogeochemical species and 7 minerals) whose evaluation required use of massively-parallel computational facilities. Modeling of a recent acetate biostimulation field experiment produced a good match to observations without specific model calibration. These results provide a dynamic picture of evolving uranium behavior during biostimulation, showing the effect of a falling water table and the transition from dominance by iron reducers to dominance by sulfate reducers. This outcome provides a rationale for using our current reactive transport model to plan upcoming field experiments at the site.